https://essopenarchive.org/doi/full/10.22541/essoar.176990453.39470985/v1

*Authors*: Ehsan Erfani

*01 February 2026*

*Abstract*
Marine low clouds exert a strong control on Earth's radiative balance, yet
their response to aerosol perturbations remains a major source of
uncertainty in climate projections and Solar Radiation Modification
strategies such as Marine Cloud Brightening (MCB). This study develops a
comprehensive framework to investigate aerosol-cloud interactions using
large-eddy simulation (LES). More than 2,200 forward Lagrangian
trajectories were constructed across the Northeast Pacific stratocumulus
deck region using satellite and reanalysis data. Principal Component
Analysis (PCA) was applied to cloud-controlling factors to objectively
select 54 representative environmental states that encompass the observed
phase space. These cases were used to initialize 48-hour, large-domain LES
(UW-SAM coupled to a prognostic aerosol scheme). The resulting LES library
reveals robust relationships between aerosol concentration, diurnal cycle
of liquid water path (LWP), mesoscale cell size, and
stratocumulus-to-cumulus transition. Systematic quantification of
model-observation biases further demonstrates strong coupling between cloud
droplet number concentration, cloud fraction (CF), and shortwave cloud
radiative effect biases, with larger errors occurring in conditions with
lower CF. In addition, higher aerosol number concentration leads to
stronger diurnal cycle of LWP and larger mesoscale cell size due to
precipitation suppression and entrainment enhancement. This framework
provides a process-level basis for evaluating aerosol perturbations and MCB
efficacy under realistic environmental conditions.

*Source: ESS Open Archive *

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