https://essopenarchive.org/doi/full/10.22541/essoar.176804689.91545166

*Authors*: Michael Diamond

*10 January 2026*

*Abstract*
Aerosol-cloud interactions exert a strong but highly uncertain negative
radiative forcing, masking current greenhouse gas-driven warming and
obscuring our ability to estimate future warming as well. ”Natural
experiments” like ship tracks have been identified as a promising means of
constraining aerosol effects on clouds; however, questions remain about the
extent to which cloud adjustments observed in ship tracks generalize to
other pollution effects. At the same time, inadvertent aerosol
perturbations like ship tracks have inspired proposals to offset global
warming impacts with deliberate aerosol cooling [e.g., marine cloud
brightening (MCB)]. Ship track aerosol are a mixture of carbonaceous
material and sulfate, but changes in fuel composition due to international
regulations have shifted aerosol composition from larger sulfate-coated to
smaller soot-dominated particles. There is currently a debate in the
literature about whether reduced cloudiness observed in some ship tracks is
due to cloud adjustments to aerosol-driven microphysical perturbations or
to aerosol absorption, which is negligible for sea salt (as would be used
for MCB). Through satellite observations both before and after these
regulations went into effect and large eddy simulation modeling of cloud
adjustments under sulfur-dominated, soot-dominated, and salt ”tracks”, we
test the hypothesis that ship tracks observed in the historical record are
good analogues for what salt tracks would behave like under MCB. If there
are large differences between sulfur and salt tracks in particular, then
current knowledge based on satellite imagery and field measurements of ship
tracks would need to be interpreted cautiously for the case of MCB and may
indeed underestimate efficacy, with implications for the merit of
small-scale outdoor perturbative studies focusing on salt tracks in
particular.

*Source: Authorea*

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