The usual suspects apply: decrease the mixing weight to 0.05 or even 0.01,
if necessary.

Happy New Year,

Marcos

2010/12/31 guohuaihong <[email protected]>

> Dear siesta community:
>
>
> I am having trouble to get a SCF calculation converged for a layered composite
> system. Can somebody give me a hand?
>
>
> Our system is "graphene n layers on top of Ni(111) surface". I am using GGA
>
> pseudopotentials for Ni and C elements. When a simplest SZ basis set is used,
>
> SCF calculation can converge. However, as it comes to the standard DZP basis
>
> set, SCF convergence becomes difficult. I don't know what to do to improve it.
>
> Here is my input file:
> ===========start of input.fdf==== ============
> SystemName         2Ni-2gra
> SystemLabel        2Ni-2gra
> NumberOfAtoms        6
> Diag.ParallelOverK   T
>
> PAO.BasisSize   DZ
>
> NumberOfSpecies      2
> %block ChemicalSpeciesLabel
>     1  28   Ni
>     2   6   C
> %endblock ChemicalSpeciesLabel
>
> LatticeConstant  2.48901587  Ang
>
> %block LatticeVectors
>   0.866025404  -0.500000     0.00000000
>   0.866025404   0.500000     0.00000000
>   0.000000000   0.000000    12.05295650
> %endblock LatticeVectors
>
> %block kgrid_Monkhorst_Pack
>   6  0  0   0.0
>   0  6  0   0.0
>   0  0  1   0.0
> %endblock kgrid_Monkhorst_Pack
>
> SpinPolarized   .false.
> XC_functional  GGA
> XC_authors     PBE
>
> %block PS.lmax
>    C   2
> %endblock PS.lmax
>
> PAO.EnergyShift   50. meV
>
> MeshCutoff        200. Ry
> DM.UseSaveDM      F
> MaxSCFiterations  200
> DM.MixingWeight   0.10
> DM.NumberPulay    3
> DM.Tolerance      0.0001
>
> MD.NumCGsteps  100
> MD.TypeOfRun   CG
> MD.UseSaveXV   T
> MD.UseSaveCG &nbsp ; F
> WriteMDXmol    F
> WriteForces    T
>
> SaveDeltaRho   F
> SaveRho        F
>
> %block GeometryConstraints
>   position from 1 to 1
> %endblock GeometryConstraints
>
> AtomicCoordinatesFormat Ang
> %block AtomicCoordinatesAndAtomicSpecies
>    1.15470054    0.000      1.6256505400   1 #Ni
>    1.73205081    0.000      2.4336003900   1 #Ni
>    1.73205081    0.000      3.2861461800   2 #C
>    2.30940108    0.000      3.2861461800   2 #C
>    2.30940108&n bsp;   0.000      4.6320596600   2 #C
>    2.88675135    0.000      4.6320596600   2 #C
> %endblock AtomicCoordinatesAndAtomicSpecies
> ===========end of input.fdf================
>
>
> Here is part of my output file:
> ===========start of output.fdf================
> .....
> siesta: iscf   Eharris(eV)      E_KS(eV)   FreeEng(eV)   dDmax  Ef(eV)
> siesta:    1    -2512.1635    -2522.5031    -2522.5031  5.9203 -7.3552
> timer: Routine,Calls,Time,% = IterSCF        1     133.954 & nbsp;82.97
> elaps: Routine,Calls,Wall,% = IterSCF        1      11.239  82.68
> siesta:    2    -2798.2370    -2503.2791    -2503.2853 15.2607  0.1093
> siesta:    3    -2514.2022    -2519.9057    -2519.9121  6.0595 -7.7756
> siesta:    4    -2513.5115    -2516.6410    -2516.6423  7.7241 -3.7334
> siesta:    5    -2598.9529    -2517.6669    -2517.6798  5.9405 -1.3577
> siesta:    6    -2541.5296    -2518.7682    -2518.7715&
> nbsp; 8.9084 -1.1456
> siesta:    7    -2604.5084    -2510.6025    -2510.6047150.0320 -0.4481
> siesta:    8    -3121.8587    -2483.1835    -2483.1859598.3458  1.7518
> siesta:    9    -2977.9663    -2491.9150    -2491.9182596.9323  4.0476
> siesta:   10    -3078.4553    -2498.1912    -2498.1984 62.3984  0.6857
> siesta:   11    -4356.4281    -2361.6155    -2361.6199609.8885-39.3225
> siesta:   12    -4489.7671    -2325.6771    -2325.6775599.9060-47.2102
> siesta :   13    -4360.2034    -2338.9801    -2338.9801600.4145-43.2638
> siesta:   14    -3448.0593    -2205.6430    -2205.6430 71.0008-56.8998
> siesta:   15    -2579.5160    -2300.5191    -2300.5276 65.1504-24.0299
> siesta:   16    -2525.8003    -2327.3343    -2327.3529 82.7621-16.0542
> siesta:   17    -2555.9318    -2346.6249    -2346.6364 48.8877-15.5471
> siesta:   18    -3513.9083    -2395.8520    -2395.8576 54.9869-12.0970
> ......
> ===========end of output.fdf================
>
> Any& nbsp;suggestion is appreciated. Thanks alot!
>
> Best wishes!
>
> HHG
>
>
>
>
>
>
> --
> Magnetism and Magnetic Materials Division
> Shenyang Materials Science National Laboratory
> Institute of Metal Research
> Chinese Academy of Sciences
> 72 Wenhua Road,Shenyang 110016, China
>
>
> +86-15140243901 (mobile)
> work:     [email protected]
>
>
>

Responder a