2016-04-05 7:25 GMT-06:00 'ST' via votca <[email protected]>:
> Hi,
>
> I'd like to coarse-grain a benzene dimer - originally solvated in a periodic
> box of water (L=29.547 Angstrom), and I want to obtain a solvent-free CG
> description (three sites per benzene molecule), generating a non-bonded pair
> potential between the sites using IBI.
>
> To keep the dimer from drifting apart, I've added a harmonic restraint
> (between centers of mass of the monomers) starting at 12 Angstrom, already
> in the full atomistic simulations.
> I'm using LAMMPS for the MD, and to keep things comparable I'd like to have
> the harmonic restraint explicitly as a spring/couple fix in the MD, rather
> than implicitly in the non-bonded potential.
> The harmonic restraint would show up in the Boltzmann inversion first guess
> at the non-bonded potential, so I thought of using a force-matching-based
> potential as an initial guess.
I think, you could simply subtract the harmonic contribution from the
Boltzmann inverted initial guess and use that one.

>
> Has anyone used VOTCA/CSG for such a case before? I could only find monomers
> in vacuum, no mention of dimers in vacuum or a large box.
> So on the one hand I tried describing the system as a single 'molecule' with
> different types of sites for each monomer, so that the non-bonded distances
> are seen as 'bonds' - in this case I can get the same distribution function
> from csg_stat and my own routine, but the potential updates seem to go
> wrong.
> On the other hand I looked at the system as two molecules with one type of
> site, but I think I am stuck there because I don't know how csg_stat
> produces the rdf in this case, so probably my way of generating the target
> distribution doesn't match and hence the IBI procedure can't get anywhere.
>
> How should I calculate the 'RDF' in this case? Given that it goes to zero at
> large distance (due to the restraint), not to one.
> Any help appreciated - please let me know if I should provide more details!
I don't see why csg_stat would work for your case, it support open
boundary conditions. You could also try to exclude the intra-molecular
contributions to rdf.

Christoph
>
> Thanks,
> ST
>
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-- 
Christoph Junghans
Web: http://www.compphys.de

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