I meant "where the drops have the concentration of ammonium acetate needed".

James


On Nov 9, 2012, at 10:06 AM, James Stroud wrote:

> This sounds like a job for ammonium acetate. Use it as your salt. Purify your 
> complex in it and then set up drops where they wells have the amount of 
> ammonium acetate needed to keep your protein stable and the wells have none, 
> or a range of concentrations. The ammonium acetate will equilibrate by vapor 
> diffusion, lowering the concentration in the drop and causing your complex to 
> come out of solution.
> 
> James
> 
> On Nov 9, 2012, at 9:14 AM, Wei Huang wrote:
> 
>> Dear CCP4BBers,
>> 
>> I have a problem in purifying protein-DNA complex for a protein that I am 
>> interested in.
>> 
>> The purification of protein only has been optimized and I've get enough 
>> yield for what I need (10 mg/2.4 L growth). And I've measured DNA binding 
>> using Fluorescence Anisotropy. The results show that my protein has the 
>> tightest binding (Kd=8 nM) to the DNA at low salt condition (30 mM KCl) in 
>> 20 mM HEPES (pH 7.5).
>> 
>> However, I came across several problems when I assemble protein-DNA complex 
>> in large scale. 
>> 
>> First, my protein is unstable at low salt condition. When I dialyzes my 
>> protein into low salt buffer (tried 30 mM and 100 mM KCl) for binding DNA, 
>> the protein precipitates. What I don't quite understand is that the DNA 
>> binding assay performed at low salt condition doesn't seem to be affected by 
>> this instability of protein. I guess it may be due to the assay was 
>> performed at very diluted protein concentration (in nM). 
>> 
>> Second, I can not purify protein-DNA complex at high salt condition with gel 
>> filtration column. Because of the first problem, I tried to assemble the 
>> complex at high salt condition (150 mM KCl, 150 mM NaCl). However, the 
>> elution profile shows no binding of DNA to my protein (no increase in the 
>> observation of protein peak and a large peak around expected position for 
>> DNA). This may be due to weaker binding at high salt as my DNA binding assay 
>> shows that the Kd under this buffer condition is ~1100 nM.
>> 
>> Third, a lot of protein is lost during dialysis of protein-DNA complex into 
>> low salt condition. I tried add DNA directly into protein in high salt 
>> buffer, then dialyze very slowly against low salt buffer. However, I still 
>> lost quite a lot of protein due to precipitation. I was able to load some 
>> sample onto the gel filtration column with low salt running buffer. And I 
>> saw the shift of protein peak in the elution profile, also protein 
>> concentration measured by Bradford assay shows that the protein 
>> concentration is much less than that expected from uv trace, suggesting the 
>> contribution to the absorbance from DNA. But the yield is very low, less 
>> than 0.2 mg of protein is left and the complex seems to be unhappy when I 
>> concentrate it. So I can not get protein sample concentrated enough for my 
>> study.
>> 
>> My previous experience with another DNA binding protein is much better. I 
>> purified it in high salt, dialyzed into low salt to binding DNA and finally 
>> purify with gel filtration column. However, the one I am currently working 
>> on seems to be very picky. If you have any suggestion regarding to my 
>> problems, I will be thankful.
>> 
>> Best regards,
>> 
>> -- 
>> Wei Huang, PhD
>> Postdoctoral Associate
>> Center for Proteomics and Bioinformatics
>> Case Western Reserve University
>> Cleveland, OH 44106
>> 
> 

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