hi ian,
yes, that aspect was in my mind, a bit, but i wanted to keep it simple. my 
point wasn't really how the "uncertainty" parameter is derived but rather its 
units. i can imagine that uncertainty in 3D could be expressed in ų (without 
helping the naïve user much) or in Å (which to me at least seems useful), but 
Ų (i.e. the B factor) seems neither logical nor helpful in this context, 
irrespective of its utility elsewhere. if you just see the B factor as a 
number, ok, you can do the √ in your head, but if it's visualized as in 
pymol/putty larger uncertainties become exaggerated – which is another word for 
"misrepresented".
cheers
j

Von: Ian Tickle <[email protected]>
Gesendet: Freitag, 28. Mai 2021 12:10
An: Hughes, Jonathan <[email protected]>
Cc: [email protected]
Betreff: Re: [ccp4bb] AW: [ccp4bb] AW: [ccp4bb] (R)MS


Hi Jonathan

On Thu, 27 May 2021 at 18:34, Hughes, Jonathan 
<[email protected]<mailto:[email protected]>> 
wrote:

 "B = 8π2<u2>  where u is the r.m.s. displacement of a scattering center, and 
<...> denotes time averaging"

Neither of those statements is necessarily correct: u is the _instantaneous_ 
displacement which of course is constantly changing (on a timescale of the 
order of femtoseconds) and cannot be measured.  So u2 is the squared 
instantaneous displacement, <u2>  is the mean-squared displacement, and so the 
root-mean-squared displacement (which of course is amenable to measurement) is 
sqrt(<u2>), not the same thing at all as u.

Incidentally, the 8π2 constant factor comes from Fourier-transforming the 
Debye-Waller factor expression I mentioned earlier.

Also for crystals at least, the averaging is not only over time, it's over all 
unit cells, i.e. the displacements are not only thermal in origin but also due 
to spatial static disorder (instantaneous differences between unit cells).


it would seem to me that we would be able to interpret things MUCH more easily 
with u rather than anything derived from u².
So then I think what you mean is sqrt(<u2>) rather than <u2>, which seems not 
unreasonable.

Cheers

-- Ian





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