Ozone is itself a greenhouse gas 

-----Original Message-----
From: [email protected]
[mailto:[email protected]] On Behalf Of Andrew Lockley
Sent: Wednesday, January 28, 2009 8:11 PM
To: Alvia Gaskill
Cc: David Schnare; [email protected]; geoengineering
Subject: [geo] Re: methane air capture


Thanks.
Is there any technical reason why a diesel engine couldn't be developed
that would reach the compression ratios needed?  I don't quite see why
it needs to be 500:1 when you only need to get it to c1800C to burn
methane.  That suggests 40:1 approx, which is doable I think.  I also
don't see why compression adjusts the ppm - surely it stays the same and
is squished.  Is that to do with supercritical fluids?

I don't think we can just throw our hands up an admit defeat if methane
outgasses on a large scale.  We have to solve the problem!

What about enhancing ozone levels to promote photchemical degradation,
or using CSP for atmospheric-pressure oxidation?

A

2009/1/29 Alvia Gaskill <[email protected]>:
> I don't think methane at ambient levels (2 ppm) can be combusted in a 
> diesel engine.  A typical diesel engine has a compression ratio of 
> around 20, meaning that the air drawn in is compressed by a factor of
20.
> http://en.wikipedia.org/wiki/Diesel_engine#How_diesel_engines_work  As

> a result, the temperature of the compressed air is raised to around 
> 1000 degrees F, high enough for the diesel fuel to autoignite.  Thus, 
> no need for spark plugs for a diesel engine.  Unfortunately, the 
> ambient concentration for autoignition of methane is about 5% or 
> around 50,000 ppm and at 1000 degrees F.  In the diesel combustion 
> chamber, it will be around 40 ppm, ambient nominally 2 ppm.  So while 
> a 5% methane in air fuel would probably burn in a diesel engine, lower
levels would not.
>
> This issue has been addressed in studies conducted for the USEPA as 
> part of the Coalbed Methane Outreach Program, run out of EPA's Climate

> Protection Division.
>
> http://www.irgltd.com/Resources/Publications/US/Technical%20and%20Econ
> omic%20Assessment%20-%20Mitigation%20of%20Methane%20Emissions%20Coal%2
> 0Mine%20Ventilation%20Air.pdf
>
> The goal of this study was to determine ways to use methane from coal 
> mine ventilation air as fuel at levels above 3000 ppm.  One of the 
> units tested was able to combust methane at levels as low as 800 ppm.

> As noted on page 3, "Below 4.5%, methane will not ignite or sustain 
> combustion on its own without a constant ignition source, unless it 
> can remain in an environment where temperatures exceed 1832 degrees F.

> Therefore, any conventional method proposed to use ventilation air as 
> a fuel or even to destroy it, would require a net energy input in 
> addition to the fuel value of the methane contained in the ventilation
air."
>
> Internal combustion engines and solar gas turbines can burn low levels

> of methane as ancillary fuel, but won't operate on ventilation gas 
> alone as the temperatures don't get high enough to combust the 
> methane.  To burn ventilation air containing methane as a primary 
> fuel, a thermal flow and a catalytic reactor were evaluated.  Both 
> require an external source of electricity to provide the initial heat 
> for combustion, with the catalytic system operating at lower 
> temperatures of around 700-1500 degrees F vs. 1832 for the other one
(page 19).
>
> So, it doesn't appear that it is possible to combust ambient levels of

> methane using a diesel engine or any other source using the methane as

> the primary fuel.  Compressing the low levels of methane in ambient 
> air to 1000 ppm, about the lower limit of the catalytic system, would 
> require a compression ratio of 500.  Even if this could be overcome, 
> in my opinion, the extremely large volumes of air required would 
> preclude the use of such a system to mitigate ambient methane.  The 
> better approach would be to limit the sources of methane emissions 
> including feedbacks to prevent a runaway outcome for which there is
also no mitigation technology.
>
>
>
> ----- Original Message ----- From: "Andrew Lockley"
> <[email protected]>
> To: "David Schnare" <[email protected]>
> Cc: <[email protected]>; "geoengineering" 
> <[email protected]>
> Sent: Wednesday, January 28, 2009 9:56 AM
> Subject: [geo] Re: methane air capture
>
>
>>
>> You don't need a licence to squash air.  I'm not proposing a fuel - 
>> I'm proposing to drive the diesel engine with windpower.
>>
>> A
>>
>> 2009/1/28 David Schnare <[email protected]>:
>>>
>>> In the U.S., use of a compresion ignition engine requires 
>>> certification of both the fuel and the engine (by EPA), and limits 
>>> the amounts of priority pollutants that may be emitted from such an 
>>> engine.  These include NOx, SOx and particulates, all of which will 
>>> emerge from the scheme you are discussing.
>>>
>>> In a regulatory state, nothing is as easy as it seems.
>>>
>>> David Schnare
>>>
>>>
>>> On Tue, Jan 27, 2009 at 8:33 PM, Andrew Lockley 
>>> <[email protected]>
>>> wrote:
>>>>
>>>> You don't need a combustible fuel-air ratio provided that the 
>>>> combustion doesn't need to be self-sustaining.  Once the correct 
>>>> temperature is reached, any methane present will oxidise.  The 
>>>> advantage of using a diesel engine is that it runs with minimal 
>>>> energy input as the temperature can be changed without 
>>>> irrecoverable energy input - the mix cools as it expands.  I 
>>>> thought about using a jet engine - essentially an adapted turboprop

>>>> or high-bypass turbofan, but I think it would be more lossy.
>>>>
>>>> I don't agree that you'd be processing 'a few hundred cc'.  I 
>>>> envisage building vast arrays of wind turbines, all connected to 
>>>> huge marine diesel engines.
>>>>
>>>> Why would you need a catalytic convertor?  The CH4 just oxidises to

>>>> H20 and Co2.  I can see the benefit of a heat exchanger, and I 
>>>> already thought of that.
>>>>
>>>> I covered the issue of hydroxl radical - it's created by ozone 
>>>> photochemistry, so the best way to manipulate it seems to be by 
>>>> delivering ozone to the stratosphere.
>>>>
>>>> A
>>>>
>>>> 2009/1/28 dsw_s <[email protected]>:
>>>> >
>>>> > Compression ignition requires a suitable ratio of fuel to air.  
>>>> > Even if compression in a diesel engine perfectly removed methane 
>>>> > from the air, you're not going to process the atmosphere a few 
>>>> > hundred cc at a time.  To remove methane from the air, I see two 
>>>> > options: increase the amount of hydroxyl radical if there's 
>>>> > enough methane to deplete it, or as you say build air-cooled CSP 
>>>> > plants.  For the CSP option you would want a counter-flow heat 
>>>> > exchanger and a catalytic converter on the outgoing air.
>>>> >
>>>> > On Jan 27, 2:03 pm, Andrew Lockley <[email protected]>
wrote:
>>>> >> If you fixed up diesel engine to a wind turbine, you'd get >> 
>>>> >> compression ignition of any methane residue in the atmosphere, 
>>>> >> even without injecting any fuel.  This would be expensive, but I

>>>> >> think it would work.
>>>> >>
>>>> >> An alternative would be to pump air through concentrated solar 
>>>> >> power plants
>>>> >>
>>>> >> Any thoughts?  We appear to need some bright ideas on methane 
>>>> >> remediation pretty soon.
>>>> >>
>>>> >> A
>>>> > >
>>>> >
>>>>
>>>> >>
>>>
>>>
>>>
>>> --
>>> David W. Schnare
>>> Center for Environmental Stewardship
>>>
>>
>> >>
>
>



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