Can someone who understands atmospheric chemistry pls  calculate
whether the ozone cure would be worse than the methane disease?

The laser idea exists already for CFCs, and I will add it to the 'ghg
remediation' wiki

A

2009/1/29 dsw_s <[email protected]>:
>
> It takes quite a bit of energy to make ozone, which then turns back
> into O2 rather quickly.
>
> Another idea for getting rid of methane is to find a wavelength it
> absorbs and the other stuff in air doesn't, then have a laser beam at
> that wavelength bounce back and forth between mirrors in the open
> air.  The excited state would have to be one that reacts readily with
> O2, or with N2 to form an intermediate that reacts with O2.  I don't
> know whether those criteria can be met effectively and affordably.
>
> --
>
> Back on my earlier suggestion of a catalytic converter --  Any time
> you heat air to combustion temperature you form NOx, so even without
> fuel you would need a catalytic converter to avoid creating
> pollution.  But the real reason for the catalytic converter in my
> suggestion is to get rid of the methane.  An internal combustion
> engine doesn't completely burn the fuel; wasted fuel is part of the
> pollution that the converter is there to remove.  So I suspect it
> would work better on methane than the compressor would.
>
> On Jan 28, 8:31 pm, "Hawkins, Dave" <[email protected]> wrote:
>> Ozone is itself a greenhouse gas
>>
>> -----Original Message-----
>> From: [email protected]
>>
>> [mailto:[email protected]] On Behalf Of Andrew Lockley
>> Sent: Wednesday, January 28, 2009 8:11 PM
>> To: Alvia Gaskill
>> Cc: David Schnare; [email protected]; geoengineering
>> Subject: [geo] Re: methane air capture
>>
>> Thanks.
>> Is there any technical reason why a diesel engine couldn't be developed
>> that would reach the compression ratios needed?  I don't quite see why
>> it needs to be 500:1 when you only need to get it to c1800C to burn
>> methane.  That suggests 40:1 approx, which is doable I think.  I also
>> don't see why compression adjusts the ppm - surely it stays the same and
>> is squished.  Is that to do with supercritical fluids?
>>
>> I don't think we can just throw our hands up an admit defeat if methane
>> outgasses on a large scale.  We have to solve the problem!
>>
>> What about enhancing ozone levels to promote photchemical degradation,
>> or using CSP for atmospheric-pressure oxidation?
>>
>> A
>>
>> 2009/1/29 Alvia Gaskill <[email protected]>:
>> > I don't think methane at ambient levels (2 ppm) can be combusted in a
>> > diesel engine.  A typical diesel engine has a compression ratio of
>> > around 20, meaning that the air drawn in is compressed by a factor of
>> 20.
>> >http://en.wikipedia.org/wiki/Diesel_engine#How_diesel_engines_work As
>>
>> > a result, the temperature of the compressed air is raised to around
>> > 1000 degrees F, high enough for the diesel fuel to autoignite.  Thus,
>> > no need for spark plugs for a diesel engine.  Unfortunately, the
>> > ambient concentration for autoignition of methane is about 5% or
>> > around 50,000 ppm and at 1000 degrees F.  In the diesel combustion
>> > chamber, it will be around 40 ppm, ambient nominally 2 ppm.  So while
>> > a 5% methane in air fuel would probably burn in a diesel engine, lower
>> levels would not.
>>
>> > This issue has been addressed in studies conducted for the USEPA as
>> > part of the Coalbed Methane Outreach Program, run out of EPA's Climate
>>
>> > Protection Division.
>>
>> >http://www.irgltd.com/Resources/Publications/US/Technical%20and%20Econ
>> > omic%20Assessment%20-%20Mitigation%20of%20Methane%20Emissions%20Coal%2
>> > 0Mine%20Ventilation%20Air.pdf
>>
>> > The goal of this study was to determine ways to use methane from coal
>> > mine ventilation air as fuel at levels above 3000 ppm.  One of the
>> > units tested was able to combust methane at levels as low as 800 ppm.
>>
>> > As noted on page 3, "Below 4.5%, methane will not ignite or sustain
>> > combustion on its own without a constant ignition source, unless it
>> > can remain in an environment where temperatures exceed 1832 degrees F.
>>
>> > Therefore, any conventional method proposed to use ventilation air as
>> > a fuel or even to destroy it, would require a net energy input in
>> > addition to the fuel value of the methane contained in the ventilation
>> air."
>>
>> > Internal combustion engines and solar gas turbines can burn low levels
>>
>> > of methane as ancillary fuel, but won't operate on ventilation gas
>> > alone as the temperatures don't get high enough to combust the
>> > methane.  To burn ventilation air containing methane as a primary
>> > fuel, a thermal flow and a catalytic reactor were evaluated.  Both
>> > require an external source of electricity to provide the initial heat
>> > for combustion, with the catalytic system operating at lower
>> > temperatures of around 700-1500 degrees F vs. 1832 for the other one
>> (page 19).
>>
>> > So, it doesn't appear that it is possible to combust ambient levels of
>>
>> > methane using a diesel engine or any other source using the methane as
>>
>> > the primary fuel.  Compressing the low levels of methane in ambient
>> > air to 1000 ppm, about the lower limit of the catalytic system, would
>> > require a compression ratio of 500.  Even if this could be overcome,
>> > in my opinion, the extremely large volumes of air required would
>> > preclude the use of such a system to mitigate ambient methane.  The
>> > better approach would be to limit the sources of methane emissions
>> > including feedbacks to prevent a runaway outcome for which there is
>> also no mitigation technology.
>>
>> > ----- Original Message ----- From: "Andrew Lockley"
>> > <[email protected]>
>> > To: "David Schnare" <[email protected]>
>> > Cc: <[email protected]>; "geoengineering"
>> > <[email protected]>
>> > Sent: Wednesday, January 28, 2009 9:56 AM
>> > Subject: [geo] Re: methane air capture
>>
>> >> You don't need a licence to squash air.  I'm not proposing a fuel -
>> >> I'm proposing to drive the diesel engine with windpower.
>>
>> >> A
>>
>> >> 2009/1/28 David Schnare <[email protected]>:
>>
>> >>> In the U.S., use of a compresion ignition engine requires
>> >>> certification of both the fuel and the engine (by EPA), and limits
>> >>> the amounts of priority pollutants that may be emitted from such an
>> >>> engine.  These include NOx, SOx and particulates, all of which will
>> >>> emerge from the scheme you are discussing.
>>
>> >>> In a regulatory state, nothing is as easy as it seems.
>>
>> >>> David Schnare
>>
>> >>> On Tue, Jan 27, 2009 at 8:33 PM, Andrew Lockley
>> >>> <[email protected]>
>> >>> wrote:
>>
>> >>>> You don't need a combustible fuel-air ratio provided that the
>> >>>> combustion doesn't need to be self-sustaining.  Once the correct
>> >>>> temperature is reached, any methane present will oxidise.  The
>> >>>> advantage of using a diesel engine is that it runs with minimal
>> >>>> energy input as the temperature can be changed without
>> >>>> irrecoverable energy input - the mix cools as it expands.  I
>> >>>> thought about using a jet engine - essentially an adapted turboprop
>>
>> >>>> or high-bypass turbofan, but I think it would be more lossy.
>>
>> >>>> I don't agree that you'd be processing 'a few hundred cc'.  I
>> >>>> envisage building vast arrays of wind turbines, all connected to
>> >>>> huge marine diesel engines.
>>
>> >>>> Why would you need a catalytic convertor?  The CH4 just oxidises to
>>
>> >>>> H20 and Co2.  I can see the benefit of a heat exchanger, and I
>> >>>> already thought of that.
>>
>> >>>> I covered the issue of hydroxl radical - it's created by ozone
>> >>>> photochemistry, so the best way to manipulate it seems to be by
>> >>>> delivering ozone to the stratosphere.
>>
>> >>>> A
>>
>> >>>> 2009/1/28 dsw_s <[email protected]>:
>>
>> >>>> > Compression ignition requires a suitable ratio of fuel to air.
>> >>>> > Even if compression in a diesel engine perfectly removed methane
>> >>>> > from the air, you're not going to process the atmosphere a few
>> >>>> > hundred cc at a time.  To remove methane from the air, I see two
>> >>>> > options: increase the amount of hydroxyl radical if there's
>> >>>> > enough methane to deplete it, or as you say build air-cooled CSP
>> >>>> > plants.  For the CSP option you would want a counter-flow heat
>> >>>> > exchanger and a catalytic converter on the outgoing air.
>>
>> >>>> > On Jan 27, 2:03 pm, Andrew Lockley <[email protected]>
>> wrote:
>> >>>> >> If you fixed up diesel engine to a wind turbine, you'd get >>
>> >>>> >> compression ignition of any methane residue in the atmosphere,
>> >>>> >> even without injecting any fuel.  This would be expensive, but I
>>
>> >>>> >> think it would work.
>>
>> >>>> >> An alternative would be to pump air through concentrated solar
>> >>>> >> power plants
>>
>> >>>> >> Any thoughts?  We appear to need some bright ideas on methane
>> >>>> >> remediation pretty soon.
>>
>> >>>> >> A
>>
>> >>> --
>> >>> David W. Schnare
>> >>> Center for Environmental Stewardship
> >
>

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