Dear Sam and Andrew,

Some problems may come up with further increasing H2. H2 is an indirect GHG.

H2 is a significant OH sink globally.

Most of the H2 is consumed in soil. In soil the following reaction takes 
place,

CO2+4H2 ? CH4+2H2O.

Furthermore, the oxidation of CH4 in the atmosphere of produces about 
half of the H2 in the atmosphere.

A good summary can be found in

http://ipcc-wg1.ucar.edu/wg1/Report/AR4WG1_Print_Ch07.pdf

Sincerely,

Oliver Wingenter





Sam Carana wrote:
> Andrew,
>
> Since hydroxyls essentially combine O and H, it may be possible to
> increase the amount of hydroxyls in the atmosphere by adding both O
> and H, although I'm unsure whether this will automatically result in
> more hydroxyls.
>
> I remember that I wrote you, back in March, that hydrogen could be
> produced and released into the atmosphere to - under the influence of
> UV light - in an effort to produce extra hydroxyl radicals, in order
> to speed up methane oxidation. If this is feasible, we should prepare
> for this as a separate geoengineering project, in order to be ready to
> dramatically increase the production of hydrogen, preferably by means
> of electrolysis powered by wind turbines, or by means of pyrolysis of
> biomass.
>
> You replied that such additional hydrogen could cause ozone depletion.
> The above process of producing hydrogen by electrolysis of water could
> at the same time produce oxygen that could be used to in turn produce
> ozone.
>
> You said you were working on a methane paper, Andrew, is this
> avialable online, or are you still working on it?
>
> Cheers!
> Sam Carana
>
>
>
> On Fri, Dec 4, 2009 at 11:53 AM, Andrew Lockley
> <[email protected]> wrote:
>   
>> In order to address the problems of ozone loss and methane excursions, we
>> need IMO to directly alter atmospheric chemistry.  Making ozone isn't
>> terribly difficult.  You can buy off-the-shelf machines which do is quite
>> happily.  If you sling them under a balloon, then they should work quite
>> merrily to boost ozone levels.  Power would be a issue, but some options
>> include microwave beams, lasers, solar panels and satellite-style
>> micro-nuclear plants.
>> I know less about hydroxyl radicals.  I'm assuming that some similar flying
>> Heath-Robinson contraptions could be used to fix them up too.  Does anyone
>> know what technologies exist, what the power, servicing, lifetime and other
>> issues are?
>> Our approach to pollution is strange.  On the ground, we're quite happy to
>> catch it, treat it and scrub it up.  We seem, however, to make little effort
>> to repair the damage in the wider environment, even when doing so doesn't
>> appear to be impossibly difficult.  Why sit back, hand-wringing, instead of
>> building some engineering solutions?
>> A
>>
>> 2009/11/15 Eugene I. Gordon <[email protected]>
>>     
>>> Andrew:
>>>
>>>
>>>
>>> Based on prior behavior I guess we might get 50 years of few or no
>>> sunspots. Hence we might have 50 years before it gets really hot. In the
>>> meantime my guess is that the Canadians and Russians will fight any attempt
>>> at Arctic geoengineering to cool or get rid of CH4. Methane conversion to
>>> CO2 is one molecule for one molecule; and CH4 is a more effective greenhouse
>>> gas so I don’t see methane conversion to CO2 as a big deal. The main
>>> converters are OH and O2H radicals formed from O3 and H2O. So means of
>>> enhancing radical formation would be desirable. Another way would be to
>>> introduce H2. All of these conversion processes are at the expense of the
>>> ozone layer.
>>>
>>>
>>>
>>> -gene
>>>
>>>
>>>
>>> From: Andrew Lockley [mailto:[email protected]]
>>> Sent: Sunday, November 15, 2009 8:41 AM
>>> To: geoengineering
>>> Subject: Re: [geo] Re: Rejected - a simple argument for SRM geoengineering
>>>
>>>
>>>
>>> At present the likely methane excursion is far from clear.  Further, it is
>>> also unclear how quickly the total excursion will occur.  The excursion rate
>>> is highly significant due to the short life of methane in the atmosphere.
>>>  The methane ends up as CO2, in itself a major issue.  However, the CO2's
>>> likely effect is nothing compared to the devastating temperature spike which
>>> may result from a sudden methane excursion.
>>>
>>>
>>>
>>> I don't oppose John's argument, but the evidence on the severity of the
>>> problem is far from conclusive.  We need much more research into:
>>>
>>> 1)  The methane reservoir in clathrates and permafrost
>>>
>>> 2) The size of potential methane sources currently frozen as organic
>>> detritus
>>>
>>> 3) The likely changes to the GWP of methane in future atmospheres, as the
>>> levels of hydroxyl radicals etc. shift over time and as a direct result of
>>> methane excursion.  Recent research on this asks more questions than it
>>> answers.
>>>
>>>
>>>
>>> My personal feeling is that the range of likely outcomes is from a
>>> significant amplification of AGW, right up to a 'Great Dying' sized
>>> mass-extinction event when we come within a sneeze of sterilising the entire
>>> planet.  I'd be tempted to bet on the latter, but I wouldn't be around to
>>> collect the winnings, so I'll keep my wallet in my pocket.
>>>
>>>
>>>
>>> My suggestions is that geoengineers look at ways to clean up the methane
>>> from the atmosphere, and then lock down the resulting carbon.  My guess is
>>> we've got about 50 years to do this, but virtually no time at all if the
>>> methane can't be dealt with once it's in the atmosphere. Therefore, I'd
>>> support John out of precautionary principle-based reasoning.
>>>
>>>
>>>
>>> A
>>>
>>> 2009/11/15 jim woolridge <[email protected]>
>>>
>>> Nice one, John; the train of argument is clear (of limpid clarity, in
>>> fact!)  The problem is that the people and institutions addressed are
>>> in the business of politics, the art of the possible, rather than in
>>> the business of logical evaluation.  They hear what you are saying and
>>> must see the validity of it. But politically what is true and what is
>>> doable do not always coincide, as we all know from as many examples as
>>> one cares to ennumerate.
>>>
>>> We have to keep hammering away at the arguments, to the point at which
>>> they are generally understood and accepted, and also keep on
>>> politicking in the sure and certain hope that eventually the
>>> acceptance of the arguments and the cowardice/caution/horse sense/
>>> opportunistic careerism of the politicos will achieve the right kind
>>> of intersection.  In the next year or so (& wouldn't it be a great
>>> help to have the environmental NGOs on board.)
>>>
>>> On Nov 12, 10:51 pm, John Nissen <[email protected]> wrote:
>>>       
>>>> It is incredible. It is so obvious.
>>>>
>>>> 1. Global warming is driven largely by atmospheric CO2 according to the
>>>> concentration above its pre-industrial level; and
>>>>
>>>> 2. After emissions are stopped it could take millenia for the
>>>> concentration to fall back to that level, because the effective lifetime
>>>> of some of that excess CO2 is many thousands of years.
>>>>
>>>> Therefore:
>>>> 3.  Drastic emissions reduction, even to zero overnight, cannot and will
>>>> not stop the Arctic continuing to warm for decades.
>>>>
>>>> Therefore:
>>>> 4. The Arctic sea ice will continue to retreat, accelerating the warming
>>>> due to the albedo effect.
>>>>
>>>> Therefore:
>>>> 5.  The permafrost will continue to thaw releasing increasing quantities
>>>> of methane, a potent greenhouse gas, potentially adding many degrees to
>>>> global warming; and
>>>>
>>>> 6.  The Greenland ice sheet will become increasingly unstable,
>>>> potentially contributing to an eventual sea level rise of 7 metres.
>>>>
>>>> Therefore:
>>>> 7.  To avoid these two catastrophes, we need to cool the Arctic quickly
>>>> enough to save the Arctic sea ice; and
>>>>
>>>> 8.  Probably the only feasible way to do this is through solar radiation
>>>> management (SRM) geoengineering.
>>>>
>>>> 9.  SRM is not a last resort, it is needed now to cool the Arctic.
>>>>
>>>> It is incredible that people do not seem to follow this train of logic -
>>>> it is so obvious.
>>>>
>>>> Yet when I challenged a panel of geoengineering experts to refute this
>>>> argument, the response was that geoengineering (even just to cool the
>>>> Arctic) was too dangerous - not that the argument was false! [1]
>>>>
>>>> So we continue to hear politicians and their advisers claiming that
>>>> emissions reduction alone can be sufficient to keep the planet safe. [2]
>>>>
>>>> And we continue to hear geoengineering experts saying that
>>>> geoengineering should only be used as a last resort. [3]
>>>>
>>>> How can this mindset be changed quickly, to avoid leaving geoengineering
>>>> too late?
>>>>
>>>> John
>>>>
>>>> P.S. Apologies to those who have heard this all before and accept the
>>>> logic as self-evident.
>>>>
>>>> [1]  This challenge was put to the panel at the launch of the Royal
>>>> Society geoengineering report, on September 1st, with response from the
>>>> team leader and panel chairman, Professor John Shepherd.
>>>>
>>>> [2]  For example at the geoengineering hearing at the House of Commons,
>>>> November 2008.
>>>>
>>>> [3] For example at the congressional hearing on geoengineering, November
>>>> 2009.
>>>>         
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