This is a great study to understand the effectiveness per unit mass *in the 
stratosphere*.  Also keep in mind that there’s an additional factor, that at 
lower altitudes it takes higher injection rates to achieve the same burden in 
the stratosphere (i.e., lower lifetime at lower injected altitude).

If the only thing you cared about was cost, then since there are existing 
studies demonstrating that you can design an aircraft to get to ~20-21km, we 
roughly know that it could be done, but higher altitude injection means less 
total sulfur injected and hence smaller side effects, and should be better 
understood both on the modeling and implementation cost as the trade may well 
be worth it.

doug

From: [email protected] <[email protected]> On 
Behalf Of Govindasamy Bala
Sent: Saturday, December 14, 2019 9:38 PM
To: Andrew Lockley <[email protected]>
Cc: geoengineering <[email protected]>
Subject: Re: [geo] Climate system response to stratospheric sulfate aerosols: 
sensitivity to altitude of aerosol layer

Dear Andrew,
Thanks for the posting. The heights studied were 16, 19 and 22 km, height that 
are relevant to solar radiation modification problem.. The final paragraph in 
the paper is worth reading to get more quantitative information from this 
modeling study.

"To summarize, for the same mass, the efficiency (defined
as changes in surface temperature per Tg S) of volcanic
aerosol is less when it is prescribed at lower altitudes in the
stratosphere (Fig. 9). For example, in our simulations, there is
a surface cooling of 0.44K for each teragram of sulfur placed
in the stratosphere at about 16 km altitude (100 hPa). There
is an additional surface cooling of 0.15K per Tg S when the
prescribed altitude is increased from about 16 km to about
22 km (37 hPa)."

On Sat, Dec 14, 2019 at 12:55 AM Andrew Lockley 
<[email protected]<mailto:[email protected]>> wrote:
Poster's note : this has significant implications for the engineering of 
delivery systems. I can't do the pressure altitude conversion in my head, but 
it's a lot higher than what's generally been planned for. We're gonna need a 
bigger boat.


https://www.earth-syst-dynam.net/10/885/2019/

Climate system response to stratospheric sulfate aerosols: sensitivity to 
altitude of aerosol layer
Krishna-Pillai Sukumara-Pillai Krishnamohan et al. Received: 01 May 2019 – 
Discussion started: 23 May 2019 – Revised: 24 Oct 2019 – Accepted: 08 Nov 2019 
– Published: 13 Dec 2019
Abstract
top<https://www.earth-syst-dynam.net/10/885/2019/#top>

Reduction of surface temperatures of the planet by injecting sulfate aerosols 
in the stratosphere has been suggested as an option to reduce the amount of 
human-induced climate warming. Several previous studies have shown that for a 
specified amount of injection, aerosols injected at a higher altitude in the 
stratosphere would produce more cooling because aerosol sedimentation would 
take longer. In this study, we isolate and assess the sensitivity of 
stratospheric aerosol radiative forcing and the resulting climate change to the 
altitude of the aerosol layer. We study this by prescribing a specified amount 
of sulfate aerosols, of a size typical of what is produced by volcanoes, 
distributed uniformly at different levels in the stratosphere. We find that 
stratospheric sulfate aerosols are more effective in cooling climate when they 
reside higher in the stratosphere. We explain this sensitivity in terms of 
effective radiative forcing: volcanic aerosols heat the stratospheric layers 
where they reside, altering stratospheric water vapor content, tropospheric 
stability, and clouds, and consequently the effective radiative forcing. We 
show that the magnitude of the effective radiative forcing is larger when 
aerosols are prescribed at higher altitudes and the differences in radiative 
forcing due to fast adjustment processes can account for a substantial part of 
the dependence of the amount of cooling on aerosol altitude. These altitude 
effects would be additional to dependences on aerosol microphysics, transport, 
and sedimentation, which are outside the scope of this study. The cooling 
effectiveness of stratospheric sulfate aerosols likely increases with the 
altitude of the aerosol layer both because aerosols higher in the stratosphere 
have larger effective radiative forcing and because they have higher 
stratospheric residence time; these two effects are likely to be of comparable 
importance.
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With Best Wishes,

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G. Bala
Professor
Center for Atmospheric and Oceanic Sciences
Indian Institute of Science
Bangalore - 560 012
India

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