Damon:

"If a peptide has an N-terminal Q or E, it will spontaneously eliminate -17
Da (-NH3) or -18 (-H2O) respectively, to form an N-terminal pyrolidone
carboxylic acid. If the N-terminal residue is C and it has been modified by
iodoacetimide, it also has an analogous reaction (-17, -NH3). Because they
are rather special (they always occur to some degree), they are the only
potential modifications that are built into X! Tandem."


On Fri, May 24, 2013 at 12:07 PM, Damon May <[email protected]> wrote:

> I'm running X! TANDEM CYCLONE TPP (2011.12.01.1) in TPP 4.6.2 on Ubuntu
> 12.04.2 LTS.
>
> Similarly to the May 17 issue posted by GATTACA, I'm seeing X!Tandem
> search results with a variable Cys modification not specified in my
> parameter files. Specifically, from the xtan.xml:
>
> <aa type="C" at="117" modified="-17.02655" />
>
> This only appears to happen on peptide n-terminal C residues, and it
> doesn't appear on all n-terminal Cysteines. This is identical behavior to
> the "quick pyrolidone" modification for Q:
>
> http://www.thegpm.org/tandem/api/pqp.html
>
> But it's happening on C as well as Q. If I run a search with this
> parameter specified:
>
>         <note type="input" label="protein, quick pyrolidone">no</note>
>
> ...then, as expected, I don't get the -17.02655 modification on n-terminal
> Q, and I also don't get it on n-terminal C.
>
> It looks to me like, most likely, the "quick pyrolidone" modification is
> erroneously (?) declaring a variable modification on n-terminal C and Q,
> rather than just Q. Can anyone verify that this is what's going on and
> indicate whether it's intended or not? If it's unintended, might there be a
> workaround other than disabling "quick pyrolidone"?
>
> Thanks,
> Damon
>
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