Hi Luis,

 thanks for the useful insight, I guess for iTRAQ(8) we need to use

<note>residue modification parameters</note>
<note type="input" label="residue, modification mass">46.9955457863@C, 
304.205360@[,304.205360@K</note> 
<note type="input" label="residue, potential modification 
mass">15.994915@M,304.205360@Y</note> 

is that correct? thanks a lot,

Alberto

El martes, 11 de octubre de 2011 20:30:27 UTC+2, Luis escribió:
>
> Hello Marcus,
> As luck would have it, I just had to conduct analysis of an iTRAQ(8) 
> sample using X!Tandem.
>
> First, there is unfortunately no GUI to set the parameters for the search, 
> at least within the TPP.
>
> Do make sure that you specify the appropriate modifications based on the 
> chemistry you used to prepare the peptides.  Other than alkylation and 
> MMTS, you should add the isobaric mass tag to all peptides -- typically at 
> the N-term as well as Lysines, but this might depend on the exact protocol 
> you followed.  Add the following to the "residue, modification mass" tag: 
> 144.102063@[,144.102063@K .  A less abundant potential modification on Y 
> might be useful to add, under "residue, potential modification mass", 
> include 144.102063@Y , as well as any other potential mods (e.g. Oxidized 
> M, etc).
>
> Also, note that the iTRAQ8-plex reagent has a very different mass 
> (304.205360), should you ever use that label.
>
> The standard xtandem/k-score parameters that we ship with the TPP already 
> exclude fragment ions lower than 125.0 Daltons; you can change this 
> parameter by adding the following line to your params file, just replace 
> the value with your desired minimum m/z:
>
> <note type="input" label="spectrum, minimum fragment mz">125.0</note>
>
> Hope this helps with your searches,
> --Luis
>
>
>
> On Mon, Sep 26, 2011 at 11:33 PM, Marcus Sjödin <[email protected] 
> <javascript:>> wrote:
>
>> Hi!
>>
>> I wish to run some iTRAQ labeled data through the TPP using the embedded 
>> search engine xtandem! The peptides have been alkylated using MMTS and 
>> labeled with the iTRAQ 4-plex (114-117). The data was acquired on a Waters 
>> Synapt using DDA mode. I have converted the .raw data to both mzML and 
>> mxXML format and thus have the data in the format ready to use for the 
>> database searching. My question regards how to define the search tandem 
>> parameter file to be set up using isobaric labeling? 
>>
>> Firstly, the default parameter file is set up for carbamidomethylation 
>> but I need to change it to MMTS which I assume just needs to be changed 
>> from 
>>
>> <note label="residue, modification mass" type="input">57.021464@C</note>
>>
>> into 
>>
>> <note label="residue, modification mass" type="input">45.987721@C</note>
>>
>>
>> But how do I define the search for iTRAQ? I assume, a mass addition for 
>> the isobaric label is needed for the MS scan as well as a exclusion of 
>> 114-117 in the MS/MS scan is needed? Is there any easy way of doing this? 
>> Is there a GUI to define the correct search settings for this that works 
>> with the xtandem in TPP? I would greatly appreciate any help on this topic!
>>
>> Sincerely, 
>> Marcus Sjödin
>>
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