I was asked by a colleague about what is expected to happen as marine bunker
fuels are desulfurized over the coming several years. My first response was
that it would reduce the SO2 emissions and so the sulfate, and since sulfate
adds to cooling, this would suggest the desulfurization would lead to a
warming influence.

But then, the key to cloud brightening is addition of CCN in relatively
unpolluted regions (so yes, over remote oceans), but is not much of the ship
traffic in relatively polluted regions? Experiments do seem to indicate that
over-saturation of CCN tends to lead to cloud clearing--so basically we are
in the Goldilocks situation--one needs to have neither too few CCN nor too
many to get cloud brightening.

So, might it be that in some polluted regions, reducing the SO2 emissions
from marine sources might actually lead to an increase in clouds/cloud
brightness? Has anyone done a really careful analysis of this? Do we really
have good quantitative estimates of what might happen? And how might all of
this play out as the other sources of SO2 are changing?

Perhaps Stephen Salter, John Latham, Alan Gadian, et al. have a paper(s) on
this that I have missed.

Mike MacCracken


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