What about the bogey of Fourier truncation ripples--I have heard many have been 
fooled by the into thinking they were seeing orbitals. How does one tell the 
difference?

JPK

-----Original Message-----
From: CCP4 bulletin board [mailto:[email protected]] On Behalf Of Phil 
Jeffrey
Sent: Thursday, February 05, 2015 3:52 PM
To: [email protected]
Subject: Re: [ccp4bb] proton scattering by X-rays

Mark,

In the small-molecule crystal structures I work with it's relatively common to 
see localized difference electron density along covalent bonds or in the places 
you'd expect to see lone pairs during refinement after you've fit and modeled 
the atoms reasonably well and the phases are pretty good.  It's usually not as 
strong as difference density for hydrogens, before you put them in, but it's 
often pretty clearly visible once you have.

(I use SHELXLE as an interface for small molecule refinements because of a 
somewhat Coot-like experience in viewing maps).

Phil Jeffrey
Princeton


> What you CAN do in fact is appropriately subtract "spherical electron 
> density" from the experimental density and see what is left (i.e.
> directional ED that is 'surplus'). I tried to quickly find a paper on 
> that, they exist, and they show that experimental density does confirm 
> what we learn in chemistry class, orbitals are not imaginary.
>
> Mark

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